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FLYCHK: Generalized population kinetics and spectral model for rapid spectroscopic analysis for all elements

TLDR
FLYCHK as discussed by the authors is a straightforward, rapid tool to provide ionization and population distributions of plasmas in zero dimension with accuracy sufficient for most initial estimates and in many cases is applicable for more sophisticated analysis.
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This article is published in High Energy Density Physics.The article was published on 2005-12-01 and is currently open access. It has received 581 citations till now.

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SPECT3D - A Multi-Dimensional Collisional-Radiative Code for Generating Diagnostic Signatures Based on Hydrodynamics and PIC Simulation Output

TL;DR: SPECT3D as discussed by the authors is a multi-dimensional collisional-radiative code used to post-process the output from radiation-hydrodynamics (RH) and particle-in-cell (PIC) codes to generate diagnostic signatures (e.g. images, spectra) that can be compared directly with experimental measurements.
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Advances in NLTE modeling for integrated simulations

TL;DR: In this paper, a simple screened-hydrogenic model was proposed to calculate ionization balance with sufficient accuracy, at a low enough computational cost for routine use in radiation-hydrodynamics codes.
References
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Rate of collisional excitation in stellar atmospheres

TL;DR: In this article, an approximate formula is proposed to compute the cross-section for excitation by electron impact for the op, where the crosssection is defined as the number of electron impacts.
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XCIII. On the theory of X-ray absorption and of the continuous X-ray spectrum

TL;DR: In this article, the theory of X-ray absorption and of the continuous Xray spectrum has been studied in the context of the XCIII theory and its application in the field of physics.
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Electron Impact Ionization Cross-Sections and Ionization Rate Coefficients for Atoms and Ions from Hydrogen to Calcium

TL;DR: In this paper, electron-impact ionization cross-sections for single ionization from the ground state are given for free atoms and for all ionization stages from hydrogen to calcium (Z=20).
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Excitation of atoms and broadening of spectral lines

TL;DR: In this article, the theory of atomic collisions between heavy particles is used to estimate cross sections of Spectral Lines, and a formula for the estimation of effective cross sections is given.
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Electron Radiative Transitions in a Coulomb Field

TL;DR: In this article, the free-free, bound-free and bound-bound Gaunt factors and oscillator strengths were computed for electrons in a pure Coulomb potential for a wide range of electron and photon energies.
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Frequently Asked Questions (18)
Q1. What are the contributions in "Flychk: generalized population kinetics and spectral model for rapid spectroscopic analysis for all elements" ?

Plasmas with arbitrary electron energy distributions, single or multiple electron temperatures can be studied as well as radiation-driven plasmas. To achieve this versatility and accuracy in a code that provides rapid response the authors employ schematic atomic structures, scaled hydrogenic crosssections and read-in tables. 

Finally, the authors are also developing a Boltzmann solver that will be integrated with FLYCHK suite to study electron energy distributions self-consistently with the population distributions of interest for a wide range of non-thermal plasma, e. g, XFEL, intense short pulse laser, and beam generated plasmas. 

For Maxwellian electron distribution, the three-body, or collisional recombinationrate coefficient is related to the ionization rate coefficient by the detailed balance as! 

For long-pulse laser-produced plasmas, such as gas bag or hohlraum experiments[28], K-shell spectroscopy and FLY have been widely used so the application of FLYCHK is straightforward. 

While the K-shell based spectroscopic code suite FLY and its predecessors [1] have been successfully employed to study hot dense plasmas for decades, the emphasis of the new plasma generation schemes are moving into uncharted regions of the temperature-density phase-space: warm dense matter, highly transient states of matter, and extremely hot and dense matter. 

A population kinetics model incorporates the results of atomic structure codes and scattering theories, plasma and statistical physics to describe atomic processes in atoms embedded in a plasma. 

The inner-shell excited levels with an n-shell electron promoted from the firstinner-shell excited level are sequentially constructed by adding the energy of bound nshell excited level with respect to its ground state to the energy of the first inner-shell excited level. 

The example the authors study is the irradiation of a solid Cu sample by a laser at 1018 W/cm3 creating a non-thermal “hot” electron distribution with a temperature of 200 keV and density of 1020 cm-3 that generate K-shell vacancies in the relatively cooler solid density Cu. 

Spectral Modeling: FLYSPECThe post-processor FLYSPEC synthesizes the emission and absorption spectra using the population distributions from the FLYCHK output file. 

There has been, and will continue to be, a resurgence in the development of novelplasma-generation techniques: x-ray lasers, ultra-short-pulse lasers, the National Ignition Facility (NIF), powerful z-pinch machines, VUV and X-ray Free Electron (XFEL) lasers. 

the spectrum using level populations of the n-based configurations from FLYCHK will in many cases fail to represent observable spectra due to the simplicity of the atomic structure and radiative transitions employed in the n-based data file. 

For the photoexcitation processes, the rate in units of s-1 is given byRij = 4! "ij J(#) d#h# $ where J(#) =1 2 I(#,µ)dµ%1+1 $where J(ν) is the mean intensity, I(ν,µ) is the specific intensity as a function of frequency ν and angle µ, and the α ij is the absorption cross-section for a transition from state i tostate j. 

This is where resonant processes by electron capture or excitation may lead to highly non-LTE distributions amongst those states. 

While the steady-state assumption is often valid for these long-pulse plasmas, in many cases one has to include the effect of opacity in both kinetics and spectrum calculations, both of which are incorporated into FLYCHK. 

This indicates the time needed for the plasma to arrive at a steady state for a given condition of Te and Ne, and provides an insight on whether the shifts and widths of K-α lines, which are generated by the hot electrons, can be usedas a time-independent diagnostic for given plasma conditions. 

(3) Collisional processesA collisional rate coefficient in units of cm3s-1 is computed with the cross-sectionσ(E) and a given electron energy distribution function fe(E) for a transition of threshold energy of ΔE as!R = Ne v" (E) fe (E)dE #E$ % ,where v is the electron velocity at energy E. 

The spontaneous emission rate from a state j to a state i is directly related to the oscillator strength, fij of the transition as! 

Then using the Van Regemorter cross-section [15] and a gaunt factor at the threshold energy Eij for σc(Eij), the authors obtain the autoionization rate as!